Femtochemistry VII Fundamental Ultrafast Processes in Chemistry Physics and Biology 1st Edition by Welford Castleman, Michele Kimble 0444528210 9780444528216

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ISBN 10: 0444528210

ISBN 13: 9780444528216

Author: A. Welford Castleman, Jr. and Michele L. Kimble

Since the emergence of femtochemistry seventeen years ago, remarkable progress has been made and femtosecond spectroscopy devoted to Chemistry and Biology has become a well established field of research, giving rise to femtochemistry and femtobiology. The significance of the field is recognized through its impact around the world, giving rise to numerous conferences which includes the most recent conference from the Femtochemistry Conference Series, Femtochemistry VII.

This title is made up of contributions made from the Femtochemistry VII conference held in Washington D.C., 17-22 July 2005. The stimulating conference was opened by Professor Ahmed Zewail (1999 Nobel Prize Winner), and as was evident by the attendees at the conference, had a very active program with the presentation of numerous talks and a large number of posters. Subjects covered include imaging, structural dynamics, and spectroscopies, fundamentals of reaction dynamics, salvation phenomenta, liquids and interfaces, aggregates/particles/surfaces, protein dynamics and photobiology, quantum control, and intense laser-matter interactions.

* Contains the most recent developments in Femtochemistry from the Femtochemistry VII conference
* Highlights the significance of femtochemistry today
* Displays extracts from the proceedings, presentations and posters from the conference

Femtochemistry VII Fundamental Ultrafast Processes in Chemistry Physics and Biology 1st Table of contents:

Part 1: Imaging, Structural Dynamics, Spectroscopies
Chapter 1: 4D Structural Dynamics
Chapter 2: Ultrafast Wave Packet, Coherent Control and Dissociation Dynamics
Chapter 3: Ultrafast laser-pump x-ray probe measurements of solvated transition metal complexes
Chapter 4: Electron dynamics of metal-carbon clusters
Chapter 5: Time resolved CARS measurements of I2 in solid Kr: vibrational state dependent dephasing times between 2.6 – 32 K
Chapter 6: The Ultrafast Photofragmentation Pathway of N, N- Dimethylisopropylamine
Chapter 7: Ultrafast photofragmentation dynamics of gas phase CH2BrCl
Chapter 8: Determination of charge state of tungsten during ultrafast hard x-ray generation
Chapter 9: Multi-dimensional fs spectroscopy of an excitonic dimer, described by Redfield relaxation theory
Chapter 10: High power synchronized femtosecond Ti: sapphire laser with sub-femtosecond timing jitter
Chapter 11: Ultrafast vibrational evolution of excited-state coumarin 153 using fs/ps CARS as a transient Raman probe
Chapter 12: Development of fs/ps CARS as a Sub-100 fs Transient Raman Probe
Chapter 13: Ultrafast fluorescence parametric amplification for femtosecond molecular dynamics research
Chapter 14: A density-functional study of the structural, electronic, and vibrational properties of Ti8Ci12 metallocarbohedrynes with relevance to ultrafast time-resolved spectroscopy

Part 2: Fundamentals of Reaction Dynamics
Chapter 15: Sub 5 fs spectroscopy of polydiacetylene
Chapter 16: Dark intermediate states in photochemical cis-trans isomerizations and pericyclic reactions
Chapter 17: Multi-component fitting of cluster dynamics
Chapter 18: Photodissociation of SO2 at 200 nm: Evidence of an anisotropy effect
Chapter 19: Energy Transfer Dynamics in Zn-Porphyrin-Appended Dendrimers
Chapter 20: Vectorial Energy Transfer: Direct Measurement of an Intermediate Transfer Step
Chapter 21: Ultrafast Dynamics of Strongly Confined Water
Chapter 22: Femtosecond-Domain Dynamical Studies of Energy-Transfer Cassettes
Chapter 23: Fluorescence of polythiophenes: the effect of intra- and interchain processes on the excited state dynamics
Chapter 24: Probing and controlling ultrafast dynamics of a molecular switch

Part 3: Solvation Phenomena
Chapter 25: Solvation and Photochemical Funnels: Environmental Effects on Conical Intersection Structure and Dynamics
Chapter 26: Simulation of resonance Raman spectra of the solvated electron in water and methanol
Chapter 27: Dynamics following charge-transfer to solvent in I- (water)n (n=3-28) clusters observed with photoelectron imaging
Chapter 28: Ultrafast Photoelectron imaging of the electronic relaxation of a molecule deposited at the surface of an argon cluster
Chapter 29: Solution Femtochemistry of Two Selected H-bonded Systems
Chapter 30: Solvent Dependent Conformational Relaxation of cis-1,3,5-Hexatriene

Part 4: Liquids and Interfaces
Chapter 31: Vibrational Echo and Pump-Probe Spectroscopic Studies of the Dynamics of Water Molecules Confined to Nanoscopic Dimensions
Chapter 32: Excited-state dynamics of the PYP chromophore in solution. Environment and structure effects
Chapter 33: Second Harmonic and Sum Frequency of Molecules at Aqueous Interfaces
Chapter 34: Solvation Dynamics in Ionic Liquids, Results from ps and fs Emission Spectroscopy
Chapter 35: Femtosecond relaxation dynamics of solvated electrons from liquid metal-ammonia solutions: Temperature jump versus local density jump
Chapter 36: Multiplex Electronic Sum Frequency Generation Spectroscopy of Dye Molecules at the Air/Water Interface
Chapter 37: Photodetachment of aqueous iodide: variation of the excitation energy and solution temperature
Chapter 38: A combined femtosecond fluorescence and TD-DFT study of uracil derivatives in aqueous solution

Part 5: Aggregates/Particles/Surfaces
Chapter 39: Ultrafast electronic and lattice processes of plasmonic nanoparticles of different shape
Chapter 40: Relaxation of photoexcited states in mass-selected Agn− and AgnO2− clusters
Chapter 41: Time-Resolved Single Molecule Spectroscopy of Conjugated Polymer Nanoparticles
Chapter 42: Influence of different anchor-bridge groups on electron transfer from the molecular chromophore perylene to the wide gap semiconductor TiO2
Chapter 43: Electron transfer from molecular chromophores to semiconductors probed with two-photon-photoemission
Chapter 44: Interfacial Electron Transfer or Concentration Quenching?

Part 6: Protein Dynamics and Photobiology
Chapter 45: Femtosecond Spectroscopy for the Study of Initial Reactions in Protein folding
Chapter 46: The photochemistry of novel flavin-binding photoreceptors
Chapter 47: Electronic 2D Spectroscopy of Light Harvesting
Chapter 48: Intermediates in the ultrafast repair of DNA by DNA photolyase
Chapter 49: Ultrafast protein dynamics
Chapter 50: A Mechanism of Photo-Labile (De)-Protection in Chemical and Biological Systems Studied by Femtosecond Vibrational Spectroscopy
Chapter 51: Photochemistry and Dynamics of Base Pairs
Chapter 52: 2D Electronic Spectroscopy of the B800-B820 LH3 Light-Harvesting Complex
Chapter 53: Spectrally Resolved Femtosecond Nonlinear Spectroscopy for the Study of Vibrational Dynamics of Carotenoid Light Harvesting Molecules
Chapter 54: Ultrafast Studies of the Electronic Structure and Dynamics of B12 Cofactors
Chapter 55: A simple artificial light harvesting dyad as a mimic of nonphotochemical quenching in green plants
Chapter 56: Ultrafast Dynamics of Fluorescent DNA Intercalators
Chapter 57: Two-photon excited-state and conformation dynamics of NADH binding with dehydrogenases
Chapter 58: Transient IR and 2D-IR spectroscopy of thiopeptide isomerization
Chapter 59: Direct observation of DNA repair by photolyase
Chapter 60: Ultrafast hydration dynamics in protein conformational transitions
Chapter 61: Intramolecular electron transfer beyond solvent control: probing sub-100 fs photoinduced electron transfer in triarylmethane lactones
Chapter 62: Fluorescence Dynamics of Coumarin on Montmorillonite Structure
Chapter 63: Fluorescence anisotropy of photoactive yellow protein (PYP) and related systems: Is the low-lying excited state of the PYP quasi-degenerate?
Chapter 64: Light-Driven Enzymatic Reaction in Thermophilic Protochlorophyllide Oxidoreductase

Part 7: Quantum Control
Chapter 65: Converting Concepts and Dreams of Coherent Control into Applications
Chapter 66: Design of circularly polarized laser pulses for periodic electron circulation in Mg-porphyrin
Chapter 67: Learning Feedback Control Analysis
Chapter 68: Analysis and Control of Ultrafast Dynamics in Clusters
Chapter 69: Controlling the dynamical pathways in the ionization processes of NaK dimers
Chapter 70: Coherent Control of Isotope Selective Ionization and Fragmentation of Potassium
Chapter 71: Understanding Learning Control in a Molecular Family
Chapter 72: Controlling the dissociative ionization of DCl by femtosecond laser pulses
Chapter 73: Spectrum Control in Femtosecond Time-Resolved Spectroscopy
Chapter 74: Pulse shaping control of spatially aligned rotational wavepackets of N2 and O2
Chapter 75: “Radiationless” photon echo
Chapter 76: Exciton Control in the FMO Complex: Influence of Laser Pulse Polarization
Chapter 77: Spin-orbit coupling under control
Chapter 78: Quantitative phase characterization and compensation by multiphoton intrapulse interference phase scan (MIIPS)

Part 8: Intense Laser – Matter Interactions
Chapter 79: Ultrafast cluster electron and Coulomb explosion dynamics driven by ultraintense laser fields
Chapter 80: Nonadiabatic multielectron dynamics in (moderaterately) strong laser fields: C60 a model case for large finite system
Chapter 81: Chirped photoelectron attochemistry
Chapter 82: Intense Femtosecond Laser Driven Explosions of Heteronuclear Clusters
Chapter 83: Spectral phase and detuning effects in high-power chirped pulse excitation of a dye solution
Chapter 84: Squeezing Rb2 wave packets with mixed adiabatic and dynamic strategies
Chapter 85: Ultrafast conformational changes in carbonmonoxy-myoglobin after photolysis observed by time-resolved circular dichroism

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Tags: Welford Castleman, Michele Kimble, Femtochemistry, Fundamental